Título:
|
Magnetic anisotropy in Cr_(2)GeC investigated by X-ray magnetic circular dichroism and ab initio calculations
|
Autores:
|
Magnuson, Martin ;
Mattesini, Maurizio
|
Tipo de documento:
|
texto impreso
|
Editorial:
|
Elsevier Science BV, 2020-05-01
|
Dimensiones:
|
application/pdf
|
Nota general:
|
info:eu-repo/semantics/openAccess
|
Idiomas:
|
|
Palabras clave:
|
Estado = Publicado
,
Materia = Ciencias: Física: Física atmosférica
,
Tipo = Artículo
|
Resumen:
|
The magnetism in the inherently nanolaminated ternary MAX-phase Cr_(2)GeC is investigated by element-selective, polarization and temperature-dependent, soft X-ray absorption spectroscopy and X-ray magnetic circular dichroism. The measurements indicate an antiferro-magnetic Cr-Cr coupling along the c-axis of the hexagonal structure modulated by a ferromagnetic ordering in the nanolaminated ab-basal planes. The weak chromium magnetic moments are an order of magnitude stronger in the nanolaminated planes than along the vertical axis. Theoretically, a small but notable, non-spin-collinear component explains the existence of a non-perfect spin compensation along the c-axis. As shown in this work, this spin distortion generates an overall residual spin moment inside the unit cell resembling that of a ferri-magnet. Due to the different competing magnetic interactions, electron correlations and temperature effects both need to be considered to achieve a correct theoretical description of the Cr_(2)GeC magnetic properties.
|
En línea:
|
https://eprints.ucm.es/60037/1/MattesiniM%2006%20preprint.pdf
|